Similar to @Acqua, I got it in this way:
Since it has to satisfy $\forall x,y \in {\Bbb R}$, it must satisfy with $x=y=0$. So this gives $C(1+0)(1+0) \geqslant 1+0 \iff C \geqslant 1$.
Also if $x=y$, then $C(1+x^{2})^{2} \geqslant 1 + (2x)^2 \iff C(1+x^{2})^{2} \geqslant 1 + 4x^2 \iff C(1+x^{2})^{2} - 4x^2 - 1 \geqslant 0 \iff C(1+x^{2})^{2} - 4(x^2 + 1) + 3 \geqslant 0$. Substituting $z = x^2 + 1 \geqslant 1, \forall x \in \Bbb R$, and since it is true $\forall z \in \Bbb R$ such that $z \geqslant 1$, implies that $Cz^2 -4z +3 \geqslant 0$ is also true.
Notice that this is a quadratic equation, and if we solve for $z$, we have: $$z = \frac{{ - ( - 4) \pm \sqrt {{{( - 4)}^2} - 4(C)(3)} }}{{2C}} = \frac{{4 \pm \sqrt {16 - 12C} }}{{2C}}$$
Since $C \geqslant 1$ and $z \in \Bbb R$ such that $z \geqslant 1 \Rightarrow$ the discriminant $d$ of the quadratic inequality is either $0$ or less than $0$ (because $16 - 12C \leqslant 0$ for some $C \in \Bbb R$). If $d$ (discriminant of the quadratic equation) is less than $0$, $z$ has complex roots. Therefore, $d=0 \Rightarrow 16 - 12C = 0 \Rightarrow C = \frac{4}{3}$.
Proof
If $C= \frac {4}{3}$, this implies that $\frac{4}{3}(1+x^2)(1+y^2) \geqslant 1 + (x+y)^2$. Using some algebra,
$$\frac{4}{3}(1+x^{2}y^{2}+x^2+y^2) \geqslant 1 + x^2 + 2xy + y^2$$
$$\frac{4}{3} + \frac{4}{3}{x^2} + \frac{4}{3}{y^2} + \frac{4}{3}{x^2}{y^2} - {x^2} - {y^2} - 2xy - 1\geqslant 0$$
$$\frac{1}{3} + \frac{1}{3}{x^2} + \frac{1}{3}{y^2} + \frac{4}{3}{x^2}{y^2} - 2xy \geqslant 0$$
$$\frac{1}{3} + \frac{1}{3}{x^2} + \frac{1}{3}{y^2} + \frac{4}{3}{x^2}{y^2} \geqslant 2xy$$
LHS is always positive and the RHS may be negative. Multiplying everything by 3, we have:
$$1 + x^2 + y^2 + 4x^{2}y^{2} \geqslant 6xy$$
$$1 + x^2 + y^2 + 2x^{2}y^{2} + 2x^{2}y^{2} \geqslant 6xy$$
$$1 + (x+y)^2 \geqslant 6xy - 2x^{2}y^{2}$$
Case 1:
If $x=o$ and $y=\text{free} \Rightarrow 1 + y^2 \geqslant 0$ (True)
Case2:
If $y=o$ and $x=\text{free} \Rightarrow 1 + x^2 \geqslant 0$ (True)
Case 3:
If $x=y \Rightarrow 1 + 4x^2 \geqslant 1 \geqslant 0 \geqslant x^{2}(6-2x^2)$(because $x^2 \geqslant 0$ and $6 - 2x^2 \leqslant 0 \Rightarrow x^{2}(6-2x^2) \leqslant 0$) (True)
Case 4:
If $x=y=0 \Rightarrow 1 \geqslant 0$ (true)
Case 5:
WLOG, if $x = \text{fixed}$ and $y = \text{variable} \Rightarrow x=a= \text{constant}$ and $1 + (a+y)^2 \geqslant 6ay-2a^{2}y^{2}$.
GRAPH: By looking at the graph, we see that this is always true.
ALGEBRAICALLY: $1 + a^2 + 2ay - 6ay + y^2 + 2a^{2}y^{2} \geqslant 0$ (moving things on the LHS). Then, when grouping: $$(1+a^2) -4ay + (1+2a^2)y^2 \geqslant 0$$. Let's check its roots:
$$\eqalign{
& y = \frac{{4a \pm \sqrt {16{a^2} - 4(1 + {a^2})(1 + 2{a^2})} }}{{2 + 4{a^2}}} \cr
& = \frac{{4a \pm \sqrt { - 4 + 4{a^2} - 8{a^4}} }}{{2 + 4{a^2}}} \cr} $$
But, the discriminant is always less than $0$. This implies that the quadratic is actually greater than $0$, i.e. $(1+a^2) -4ay + (1+2a^2)y^2 > 0$
Q.E.D.