You made a mistake in squaring the right hand side:
$$
(3-3t)^2=9-18t+9t^2
$$
However you have also to impose the condition $3-3t\ge0$, because the left hand side is non negative by definition. So you get
$$
9t^2-22t+8=0,\qquad t\le1
$$
The quadratic equation has roots $2$ and $4/9$, as it's easy to see. Hence the unique solution to your equation is $t=4/9$.
If you "back substitute", you can understand what happens: for $t=2$ the left hand side is $\sqrt{4\cdot2+1}=3$, while the right hand side is $3-3\cdot2=-3$.
For $t=4/9$, the left hand side is $\sqrt{16/9+1}=5/3$, and the right hand side is $3-3\cdot(4/9)=3-4/3=5/3$.
The problem is that upon squaring you also add the solutions to $\sqrt{4t+1}=-(3-3t)$ that is another equation.