From hypergeometric function to elliptic integrals
The hypergeometric function $_3F_2$ from your link (or user17762's answer) may be rewritten (using following integral representation and $_2F_1\left(1,1;\frac32; t\right)=\frac d{dt}\left[\left(\arcsin\sqrt{t}\,\right)^2\right]$) as :
\begin{align}
\tag{1}I&=\;_3F_2\left(1,1,1;\frac32,\frac32;\frac1{16}\right)=\frac 12\int_0^1\frac{_2F_1\left(1,1;\frac32;\frac x{16}\right)}{\sqrt{1-x}}dx\\
&=2\int_0^1\frac{\arcsin\frac{\sqrt{x}}4}{\sqrt{x\,(1-x)\left(1-\frac x{16}\right)}}dx\\
\tag{2}&=16\int_0^{1/4}\frac{\arcsin u}{\sqrt{(1-16 u^2)\left(1-u^2\right)}}\,du\\
&\tag{3}=16\int_0^{\arcsin(1/4)} \frac {y}{\sqrt{1-4^2\sin(y)^2)}}\;dy\\
&=\left.16\;y\;F\left(y, 4\right)\right|_0^{\arcsin(1/4)}-16\int_0^{\arcsin(1/4)}\;F\left(y, 4\right)\;dy\\
\tag{4}&=4\;\arcsin(1/4)\;K\left(\frac 1{4}\right)-16\int_0^{\arcsin(1/4)}\;F\left(y, 4\right)\;dy\\
\end{align}
With $\;\displaystyle F(\phi,k):=\int_0^{\phi} \frac {dy}{\sqrt{1-k^2\sin(y)^2)}},\;K(k):=F\left(\frac{\pi}2,k\right)\;$ the incomplete and complete elliptic integral of the first kind $F$ and $K$ (one should take care of replacing $F(\phi,k)$ by EllipticF[$\phi,k^2$] and $K(k)$ by EllipticK[$k^2$] while using Alpha/Mathematica).
'$I$' may be expressed with elliptic integrals but this doesn't seem to help for a closed form... Observing that $\;\displaystyle K\left(\frac 1{4}\right)=\frac{\pi}2\sum_{k=0}^\infty\frac{\binom{2k}{k}^2}{2^{8\,k}}\;$ let's start it all again using the
Squared central binomial series
We want $\;\displaystyle I=\sum_{k=0}^\infty \frac 1{(2k+1)^2\binom{2k}{k}^2}\;$ but Nected Batir proved in 2004 following more general formula (for $n\in\mathbb{N},\; n\ge3$) :
\begin{align}
\tag{5}I_n(x)&:=\sum_{k=0}^\infty \frac{x^{2k+1}}{(2k+1)^n\,\binom{2k}{k}^2}\\
&=\frac{4\,(-1)^{n-3}}{(n-3)!}\int_0^{\pi/2}\int_0^{\arcsin(x\cos(y)/4)}\frac t{\sin(t)}\;\log^{n-3}\left(\frac{4\sin(t)}{x\cos(y)}\right)\;dt\,dy\\
\end{align}
For $\,n=3\,$ this is simply
$\;\displaystyle I_3(x)=\int_0^{\pi/2}\int_0^{\arcsin(x\cos(y)/4)}\frac t{\sin(t)}\;dt\,dy\;\;$ and after derivation
\begin{align}
I_2(x)&=x\,I_3(x)'=4\,x\int_0^{\pi/2} \frac {\arcsin(x\cos(y)/4)}{x\cos(y)/4} \frac {\partial}{\partial x}\left[\arcsin(x\cos(y)/4)\right]\;dy\\
\tag{6}I_2(x)&=4\int_0^{\pi/2} \frac {\arcsin(x\cos(y)/4)}{\sqrt{1-(x\cos(y)/4)^2}} \;dy\\
\end{align}
Unfortunately this is merely $(2)$ in the case $x=1$ (the integral for $x=4$ is divergent and $I_3(4)=8\pi G-14\zeta(3)\;$ but this won't help here...) so nothing complete here either...
The journey may be of interest anyway...